A Protometabolic One-Pot Synthesis of Orotate and Pyruvate

Department, Center, or Institute

Chemistry

Presentation Format

Department Organized Oral Session

Presentation Type

On-campus research

Description

A reaction between two glycine derivatives generates both the nucleobase orotate, a precursor of biological pyrimidines, and pyruvate, a core metabolite in the citric acid cycle and amino acid biosynthesis. The reaction proceeds in water at mild pH and temperature to provide significant yields of the two widely divergent chemical motifs. Thio substitution within the orotate ring enables the generation of nucleoside derivatives. The identification of compatible reactants and conditions that provide multiple building blocks may increase the plausibility of complex biopolymers emerging early in a protometabolism.

Department Organized Oral Session Title

Undergraduate Chemistry Research

Moderator/Professor

Timothy Hanks, Chemistry

Session Number

3

Start Date and Time

4-9-2019 1:45 PM

Location

Patrick Lecture Room, Plyler Hall 126

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Apr 9th, 1:45 PM

A Protometabolic One-Pot Synthesis of Orotate and Pyruvate

Patrick Lecture Room, Plyler Hall 126

A reaction between two glycine derivatives generates both the nucleobase orotate, a precursor of biological pyrimidines, and pyruvate, a core metabolite in the citric acid cycle and amino acid biosynthesis. The reaction proceeds in water at mild pH and temperature to provide significant yields of the two widely divergent chemical motifs. Thio substitution within the orotate ring enables the generation of nucleoside derivatives. The identification of compatible reactants and conditions that provide multiple building blocks may increase the plausibility of complex biopolymers emerging early in a protometabolism.